Volume 46 Issue 5
Jun.  2017
Turn off MathJax
Article Contents

Song Yinglin, Li Zhongguo. Ultrafast nonlinear refractive effect and mechanism of solvent nitrobenzene[J]. Infrared and Laser Engineering, 2017, 46(5): 502001-0502001(5). doi: 10.3788/IRLA201746.0502001
Citation: Song Yinglin, Li Zhongguo. Ultrafast nonlinear refractive effect and mechanism of solvent nitrobenzene[J]. Infrared and Laser Engineering, 2017, 46(5): 502001-0502001(5). doi: 10.3788/IRLA201746.0502001

Ultrafast nonlinear refractive effect and mechanism of solvent nitrobenzene

doi: 10.3788/IRLA201746.0502001
  • Received Date: 2017-05-01
  • Rev Recd Date: 2017-05-10
  • Publish Date: 2017-05-25
  • The third-order nonlinear refractive index n2 of nitrobenzene liquid was studied using Z-scan technique under femtosecond and picosecond laser pulses. The Z-scan results demonstrate that the n2 value under 20 ps, 532 nm laser pulse excitation is 11 times larger than that under 300 fs, 800 nm excitation. The mechanism of nonlinear refraction dynamics of nitrobenzene was investigated using pumpprobe with phase object technique under femtosecond pulses excitation. The nonlinear response function of nitrobenzene under ultrafast laser excitation was determined from the pump-probe experimental results. The target of the present work is to provide a reference for future work of integrated photonic device and nonlinear optical measurement based on solvent nitrobenzene.
  • [1] Mcmorrow D, Lotshaw W T, Kenneywallace G A, et al. Femtosecond optical Kerr studies on the origin of the nonlinear responses in simple liquids[J]. IEEE Journal of Quantum Electronics, 1988, 24(2):443-454.
    [2] Dini D, Calvete M J F, Hanack M. Nonlinear optical materials for the smart filtering of optical radiation[J]. Chemical Reviews, 2016, 116(22):13043-13233.
    [3] Kong D, Ao G, Gao Y, et al. Ultrafast third-order optical nonlinearities in DMSO[J]. Chinese Optics Letters, 2012, 10(11):111601-111601.
    [4] Hafizi B, Palastro J P, Penano J R, et al. Stimulated Raman scattering and nonlinear focusing of high-power laser beams propagating in water[J]. Optics Letters, 2015, 40(7):1556-1558.
    [5] Si J, Hirao K. Phase-matched second-harmonic generation in cross-linking polyurethane films by thermal-assisted optical poling[J]. Applied Physics Letters, 2007, 91(9):091105.
    [6] Tan W, Liu H, Si J, et al. Control of the gated spectra with narrow bandwidth from a supercontinuum using ultrafast optical Kerr gate of bismuth glass[J]. Applied Physics Letters, 2008, 93(5):051109.
    [7] Kedenburg S, Gissibl T, Steinle T, et al. Towards integration of a liquid-filled fiber capillary for supercontinuum generation in the 1.2-2.4m range[J]. Optics Express, 2015, 23(7):8281-8289.
    [8] Kieu K, Schneebeli L, Norwood R A, et al. Integrated liquid-core optical fibers for ultra-efficient nonlinear liquid photonics[J]. Optics Express, 2012, 20(7):8148-8154.
    [9] Ferdinandus M R, Reichert M, Ensley T R, et al. Dual-arm Z-scan technique to extract dilute solute nonlinearities from solution measurements[J]. Optical Materials Express, 2012, 2(12):1776-1790.
    [10] Van Steerteghem N, Clays K, Verbiest T, et al. Third-harmonic scattering for fast and sensitive screening of the second hyperpolarizability in solution[J]. Analytical Chemistry, 2017, 89(5):2964-2971.
    [11] Reichert M, Hu H, Ferdinandus M R, et al. Temporal, spectral, and polarization dependence of the nonlinear optical response of carbon disulfide[J]. Optica, 2014, 1(6):436-445.
    [12] Zhong Q, Fourkas J T. Optical Kerr effect spectroscopy of simple liquids[J]. Journal of Physical Chemistry B, 2008, 112(49):15529-15539.
    [13] Iliopoulos K, Potamianos D, Kakkava E, et al. Ultrafast third order nonlinearities of organic solvents[J]. Optics Express, 2015, 23(19):24171-24176.
    [14] Miguez M L, De Souza T G B, Barbano E C, et al. Measurement of third-order nonlinearities in selected solvents as a function of the pulse width[J]. Optics Express, 2017, 25(4):3553-3565.
    [15] Li Y, Kuo Y, Huang P, et al. Thermal lensing effect of CS2 studied with femtosecond laser pulses[J]. Physical Chemistry Chemical Physics, 2015, 17(38):24738-24747.
    [16] Yan X, Zhang X, Shi S, et al. Third-order nonlinear susceptibility tensor elements of CS 2 at femtosecond time scale[J]. Optics Express, 2011, 19(6):5559-5564.
    [17] Shelton D P. Orientation correlation and local field in liquid nitrobenzene[J]. Journal of Chemical Physics, 2016, 144(23):234506.
    [18] Wu H, Song Y, Yu G, et al. Transient grating study of the intermolecular dynamics of liquid nitrobenzene[J]. Chinese Physics B, 2016, 25(10).
    [19] Yang J, Song Y, Wang Y, et al. Time-resolved pump-probe technology with phase object for measurements of optical nonlinearities.[J]. Optics Express, 2009, 17(9):7110-7117.
    [20] Zhao P, Reichert M, Hagan D J, et al. Measurement of nonlinear optical response functions of common organic solvent[C]//Optical Society of America, 2016:JW2A-54.
  • 加载中
通讯作者: 陈斌, bchen63@163.com
  • 1. 

    沈阳化工大学材料科学与工程学院 沈阳 110142

  1. 本站搜索
  2. 百度学术搜索
  3. 万方数据库搜索
  4. CNKI搜索

Article Metrics

Article views(505) PDF downloads(174) Cited by()

Related
Proportional views

Ultrafast nonlinear refractive effect and mechanism of solvent nitrobenzene

doi: 10.3788/IRLA201746.0502001
  • 1. Department of Physics,Harbin Institute of Technology,Harbin 150001,China;
  • 2. College of Physics & Electronic Engineering,Changshu Institute of Technology,Changshu 215500,China

Abstract: The third-order nonlinear refractive index n2 of nitrobenzene liquid was studied using Z-scan technique under femtosecond and picosecond laser pulses. The Z-scan results demonstrate that the n2 value under 20 ps, 532 nm laser pulse excitation is 11 times larger than that under 300 fs, 800 nm excitation. The mechanism of nonlinear refraction dynamics of nitrobenzene was investigated using pumpprobe with phase object technique under femtosecond pulses excitation. The nonlinear response function of nitrobenzene under ultrafast laser excitation was determined from the pump-probe experimental results. The target of the present work is to provide a reference for future work of integrated photonic device and nonlinear optical measurement based on solvent nitrobenzene.

Reference (20)

Catalog

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return